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Tuning phenoxyl-substituted diketopyrrolopyrroles from quinoidal to biradical ground states through (hetero-)aromatic linkers

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Posted January 21st, 2021 by admin

Chem. Sci., 2021, 12,793-802DOI: 10.1039/D0SC05475E, Edge Article Open Access &nbsp This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Rodger Rausch, Merle I. S. Röhr, David Schmidt, Ivo Krummenacher, Holger Braunschweig, Frank WürthnerBy variation of spacer aromaticity, a spin crossover from thienylene/furylene-linked quinones DPP2q/DPP3q to phenylene-bridged biradical DPP1?? (y0 = 0.75) with a singlet open shell ground state (?EST = 19 meV) was achieved.The content of this RSS Feed (c) The Royal Society of Chemistry

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