A Flexible, Redox-Active Macrocycle Enables the Electrocatalytic Reduction of Nitrate to Ammonia by a Cobalt Complex

Chem. Sci., 2018, Accepted ManuscriptDOI: 10.1039/C8SC00721G, Edge Article Open Access &nbsp This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Song Xu, Daniel Ashley, Hyuk-Yong Kwon, Gabrielle Ware, Chun-Hsing Chen, Yaroslav Lozovyy, Xinfeng Gao, Elena Jakubikova, Jeremy M. SmithThe cobalt macrocycle complex [Co(DIM)Br2]+ (DIM = 2,3-dimethyl-1,4,8,11- tetraazacyclotetradeca-1,3-diene) is an electrocatalyst for the selective reduction of nitrate to ammonia in aqueous solution. The catalyst operates over a wide pH...The content of this RSS Feed (c) The Royal Society of Chemistry

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